Origin of resonant Raman excitation profiles red-shifted from optical absorption profiles

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Abstract

We observe that the Raman excitation profile in matrix-isolated Br2 is significantly red-shifted from the absorption maximum and show that a straightforward relationship between the two can in general not be expected. A simple theory considering only the resonant contributions describes our data reasonably well. In addition, we discuss the effect on our results of interference between the B and Π1u1 states.

Original languageEnglish (US)
Pages (from-to)1610-1613
Number of pages4
JournalPhysical Review Letters
Volume37
Issue number24
DOIs
StatePublished - Jan 1 1976
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy(all)

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